Zoids—powerful animal-shaped combat mechs—are no longer used in warfare, but in organized sporting competitions. The Blitz Team, a group of pilots struggling to carve out a niche for themselves in the Zoid battling leagues, experience a stroke of luck when Bit Cloud, a vagrant junk dealer, wanders into their midst and proves himself capable of piloting the temperamental Liger Zero, a Zoid that refuses to let anyone else into its cockpit. Led by Bit and the Liger, the Blitz Team steadily make their way to the top—but along the way they attract the unwelcome attention of the Backdraft Group, an organization of Zoid pilots that operates outside the laws set down by the Zoid Battle Commission. The Backdraft want powerful Zoids to add to their ranks, and they have their eye on the Liger Zero...

Although already a third-year high school student, Rikka Takanashi remains a chuunibyou—a "disease" that causes people to fantasize about themselves and their surroundings. Her relationship with Yuuta Togashi has also gone unchanged for the past six months, and with entrance exams right around the corner, both of them strive to enroll at the same college. However, Tooka—Rikka's elder sister—decides to take Rikka to Italy as she has found a stable job there. This unforeseen turn of events causes a commotion between the couple as neither of them want to be separated from each other. Desperate for ideas, they seek assistance from their friends, and after a brief conversation, they come up with a plan—to elope. Chuunibyou demo Koi ga Shitai! Movie: Take On Me is a sensational drama featuring the couple—Yuuta and Rikka—as they journey across Japan. The two attempt to prevent Rikka from being taken to Italy, but will they be able to succeed in doing so?

On an archaelogical mission to the end of the known universe, Professor Daiba unwitting unleashes an ancient horror from its confines. Five years later the malevolent alien force sets in motion a plan which reunites the various crewmembers of the Arcadia to sail the stars once more as well as bring Tadashi Daiba to meet Harlock for the first time (again).

A VHS only special episode. Also known as Episode 95.